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L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Aging and free volume in polymers of intrinsic microporosity (PIM) S. Harms, K. Rätzke, F. Faupel, N. Chaukura, P. M. Budd W. Egger, L. Ravelli Accepted for publication, Journal of Adhesion (01/2012)
New insights into the microencapsulation properties of sodium caseinate and hydrolysed casein Drusch, S., Serfert, Y., Berger, A., Shaikh, M.Q., Rätzke, K., Zaporojtchenko, V., Schwarz, K.
Food Hydrocolloids 27 (2012) 332-338
Structural investigation on functionalized 6FDA-copolyimide films R. Konietzny, C. Barth, S. Harms, K. Rätzke, P. Kölsch, C. Staudt Polymer International, 60 (12) (2011) 1670-1678
Reactive epoxies with functional zeolite fillers: IR spectroscopy and PALS studies M. Q. Shaikh, K. Rätzke, J. Ch. Gaukler, W. Possart, F. Faupel Journal Materials Research 26, (22) (2011) 2877-2886
Gas transport and free volume in hexafluoropropylene polymers N.A. Belov, A.A.Zharov, A.V.Shashkin, M.Q.Shaikh K.Raetzke, Yu.P.Yampolskii Journal of Membrane Science, 383 (2011) 70– 77
Free volume distribution at the Teflon AF/Si interfaces probed by a slow positron beam S. Harms, K. Rätzke, V. Zaporojtchenko, F. Faupel W. Egger, L. Ravelli Polymer, 52 (2011) 505
Free Volume Changes on Optical Switching in Azobenzene-Polymethylmethacrylate Blends Studied by a Pulsed S. Harms, K. Rätzke, C. Pakula, V. Zaporojtchenko. Th. Strunskus, F. Faupel, W. Egger, P. Sperr journal polymer science, part B: polymer physics 49 (6) (2011) 404
Free volume studies of interphases in model nanocomposites by positron annihilation lifetime spectroscopy S. Harms, K. Rätzke, F. Faupel, G. Schneider, L. Wöllner, D. Richter Macromolecules, 43 (2010) 10505
Metallische Gläser - Hart im Nehmen und extrem vielseitig L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Welt der Physik www.weltderphysik.de/de/8475.php (2010)
Molecular dynamics approach to structure-property correlation in epoxy resins for thermo-mechanical lifetimemodeling B. Wunderle, E. Dermitzaki, O. Hölck, J. Bauer, H. Walter, Q. Shaikh, K. Rätzke, F. Faupel, B. Michel, H.
Reichl Microelectronics Reliability 50, 7 (2010) 900-909
Diffusion and viscous flow in bulk glass forming alloys A. Bartsch, V. Zöllmer, K. Rätzke, A. Meyer, F. Faupel Invited review, Journal of Alloys and Compounds 509S, Supplement 1, (2011), S2-S7
Subnanometre size free volumes in amorphous Verapamil hydrochloride: A positron lifetime and PVT studythrough Tg in comparison with dielectric relaxation spectroscopy G. Dlubek; M. Q. Shaikh, K. Rätzke, J. Pionteck, M. Paluch, F. Faupel European Journal of Pharmaceutical Sciences, 41 (2010) 388
Free volume from positron lifetime and pressure-volume-temperature experiments in relation to structuralrelaxation of van der Waals molecular glass-forming liquids G. Dlubek, M. Q. Shaikh, K. Rätzke, M. Paluch, and F. Faupel Journal of Physics: Cond. Matter, 22 (2010) 235104
The Free volume investigation of polymers of intrinsic microporosity (PIMs). PIM-1 and a PIM1 copolymer withincreased stiffness T. Emmler, K. Heinrich, D. Fritsch, P. M. Budd, N. Chaukura, D. Ehlers, K. Rätzke, F. Faupel Macromolecules, 43 (2010) 6075
Dynamic arrest in multicomponent glass forming alloys A. Bartsch, K. Rätzke, A. Meyer, F. Faupel Phys. Rev. Lett., 104 (2010) 195901
Free volume and swelling in thin films of poly(N-isopropylacrylamide) end-capped with n-butyltrithiocarbonate S. Harms, K. Rätzke, F. Faupel, W. Egger, L. Ravello, A. Laschewsky, W. Wang, P. Müller-Buschbaum Macromolecular Rapid Communications, 31 (2010) 1364
Open volume in bioadhesive detected by positron annihilation lifetime spectroscopy K. Rätzke, M. Wiegemann, M. Q. Shaikh, S. Harms, R. Adelung, W. Egger, P. Sperr L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Acta Biomaterialia, 6 (2010) 2690-2694
Shelf stability of reactive adhesive formulations: a case study for dicyandiamide-cured epoxy system K. Rätzke, M. Q. Shaikh, F. Faupel, P.-L. M. Noeske International Journal of Adhesion & Adhesives, 30 (2010) 105–110
Molecular Dynamics Simulation and Mechanical Characterisation for the Establishment of Structure-PropertyCorrelations for Epoxy Resins in Microelectronics Packaging Applications B. Wunderle, E. Dermitzaki, O. Holck, J. Bauer, H. Walter, M.Q. Shaikh, K. Rätzke, F. Faupel, B. Michel Editors: L. J. Ernst, G. Q. Zhang, W. D. VanDriel, P. Rodgers, C. Bailey, O. deSaintLeger EXPERIMENTS IN MICRO-ELECTRONICS AND MICRO-SYSTEMS, 10th International Conference onThermal, Mechanical and Multi-Physics Simulation and Experiments Condensable gas permeation in poly(amide-b-ethylene oxide)/polyethylene glycol blend membranes and itscorrelation with free volume W. Yave, A. Car, K.-V. Peinemann, M. Q. Shaikh, K. Rätzke, F. Faupel Journal of Membrane Science, 339 (2009) 177-183
The temperature dependence of free volume in phenyl salicylate and its relation to structural dynamics: Apositron annihilation lifetime and pressure-volume-temperature study G. Dlubek, M. Q. Shaikh, K. Rätzke, F. Faupel, J. Pionteck, M. Paluch J. Chem. Phys., 130 (2009) 144906
Molecular Dynamics Approach to Structure-Property Correlation in Epoxy Resins for Thermo-MechanicalLifetime Modeling B. Wunderle, E. Dermitzaki, O. Holck, J. Bauer, H. Walter, M.Q. Shaikh, K. Rätzke, F. Faupel, B. Michel H.
Reichl IEEE 59TH ELECTRONIC COMPONENTS AND TECHNOLOGY CONFERENCE, 59th ElectronicComponents and Technology Conference MAY 26-29, 2009 San Diego, CA Differences in free volume elements of the carrier matrix affect the stability of microencapsulated lipophilic foodingredients S. Drusch, K. Rätzke, M. Q. Shaikh, Y. Serfert, H. Steckel, M. Scampicchio, I. Voigt, K. Schwarz, S. Mannino Food Biophysics, 4 (2009) 42-48
L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
A pressure-volume-temperature and positron lifetime study G. Dlubek, J. Pionteck, K. Rätzke, J. Kruse, F. Faupel Macromolecules, 41 (2008) 6125-6133
The temperature dependency of the free volume from positron lifetime experiments and its relation to structuraldynamics: Phenylphthalein-dimethylether G. Dlubek, M. Q. Shaikh, K. Rätzke, F. Faupel, M. Paluch Phys. Rev. E, 78 (2008) 051505
Temperature dependence of positron annihilation lifetimes in high permeability polymers: amorphous TeflonsAF M. Rudel, J. Kruse, K. Rätzke, F. Faupel, Y. P. Yampolskii, V. P. Shantarovich, G. Dlubek Macromolecules, 41 (2008) 78
Free volume in C-60 modified PPO polymer membranes by positron annihilation lifetime spectroscopy J. Kruse, K. Rätzke, F. Faupel, D. M. Sterescu, D. F. Stamatialis, M. Wessling J. Phys. Chem. B, 111 (2007) 13914 –13918
Unusual Temperature Dependence of the Positron Lifetime in a Polymer of Intrinsic Microporosity R. De Miranda, J. Kruse, K. Rätzke, F. Faupel, D. Fritsch, V. Abetz, P. M. Budd, J. D. Selbie, N. B. McKeown,B. S. Ghanem Phys. Stat. Sol. Rapid Res. Lett., 5 (2007) 190
Diffusion in bulk glass forming alloys – from the glass to the equilibrium melt K. Rätzke, V. Zöllmer, A. Bartsch, A. Meyer, F. Faupel Defect and Diffusion Forum, 66 (2007) 109
Boltorn-modified poly(2,6-dimethyl-1,4phenylen oxide) gas separation membranes D. Sterescu, D. F. Stamatialis, E. Mendes, J. Kruse, K. Rätzke, F. Faupel, M. Wessling Macromolecules, 40 (2007) 5400
Codiffusion of 32P and 57Co in glass-forming Pd43Cu27Ni10P20 alloy and its relation to viscosity A. Bartsch, K. Rätzke, F. Faupel, A. Meyer Appl. Phys. Lett., 89 (2006) 121917
L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Radiotracer diffusion measurements of noble metal atoms in semiconducting organic films M. Scharnberg, J. Kanzow, K. Rätzke, R. Adelung, S. Meyer, J. Pflaum, F. Faupel in: Organic thin-film electronics, Editors A.C. Arias, N. Tessler, L. Burgi, and J.A. Emerson Mater. Res. Soc. Symp. Proc. 871E, Warrendale, PA (2005)
Free Volume in Polyimides: Positron Annihilation Experiments and Molecular Modelling J. Kruse, J. Kanzow, K. Rätzke, F. Faupel, M. Heuchel, J. Frahn, D. Hofmann Macromolecules, 38 (2005) 9638
Ag-diffusion in the organic semiconductor Diindenoperylene M. Scharnberg, J. Hu, , J. Kanzow, K. Rätzke, R. Adelung, F. Faupel, J. Pflaum Defect and Diffusion Forum, 237-240 (2005) 993
Free volume in polymeric membranes: Experiment and simulation J. Kruse, J. Kanzow, K. Rätzke, F. Faupel, M. Heuchel, J. Frahn, D. Hofmann invited paper, Membrane News, 66 (2004) 51
Radiotracer measurements as a sensitive tool for the detection of metal penetration in molecular-based organicelectronics M. Scharnberg, J. Hu, J. Kanzow, K. Rätzke, R. Adelung, F. Faupel, C. Pannemann, U. Hilleringmann, S. Meyer,J. Pflaum Appl. Phys. Lett., 86 (2005) 024104
Diffusion in bulk metallic glass forming Pd-Cu-Ni-P alloys: from the glass to the equilibrium melt K. Rätzke, V. Zöllmer, A. Bartsch, A. Meyer, F. Faupel invited review, Liquid and amorphous Metals LAM 12, Metz
Journal of Non-Crystalline Solids, 353 (32) (2007) 3285
Diffusion in metallic glasses and undercooled metallic melts Z. Metallkunde, 95 (2004) 956
Zr65Al7.5Ni10Cu17.5 in its amorphous and supercooled liquid states studied by A.Dhawan, K. Rätzke, F. Faupel, S. K. Sharma L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
phys. stat. sol. (a), 199 (2003) 431
Structrual investigations of rare-earth doped PbTiO3 thin films Mat. Sci. Eng. B, 113 (2004) 259
Quenching rate dependence of free volume in a Zr-Cu-Ni-Ti-Be glass as probed by positron annihilation lifetimespectroscopy A. Rehmet, K. Günther-Schade, K. Rätzke, U. Geyer, F. Faupel phys. stat. sol. (a), 201 (2004) 467
Diffusion and isotope effect in bulk metallic glass forming Pd-Cu-Ni-P alloys from the glass to the equilibriummelt J. Mat. Res., 18 (2003) 2688
Free volume evolution in bulk metallic glass during high temperature creep B. S. S. Daniel, M. Heilmaier, B.Bartusch, J. Kanzow, K. Günther-Schade, K. Rätzke, J. Eckert, F. Faupel MRS Symp. Proc., 754 (2003) 11.16
Diffusion in a metallic melt at the critical temperature of mode coupling theory V. Zöllmer, A. Meyer, K. Rätzke, F. Faupel Phys. Rev. Lett., 92 (2003) 195502-1
Biegeeigenschaften fünf ausgewählter Ni-Ti Bogenmaterialen der Dimension 0.016"x0.022" H. Fischer-Brandies, M. Es-Souni, N. Kock, K. Raetzke, O. Bock Fortschritte der Kieferorthopädie, 64 (2003) 88
Diffusion in metallic glasses and supercooled melts Chapter 6 in: Diffusion in Condensed Matter, Editors. P. Heitjans, J. Kärger, revised edition, Springer Verlag
Silver diffusion in Fe40Ni38Mo4B18 metallic glass under high vacuum S. Lenser, S. Daniel, V. Zöllmer, J. Erichsen K. Rätzke, S. Deki, F. Faupel L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Scripta Mater., 48 (2003) 275
Diffusion in metallic glasses and supercooled melts F. Faupel, W. Frank, M.-P. Macht, H. Mehrer, V. Naundorf, K. Rätzke, H. R. Schober, S. K. Sharma, H.
Teichler Review of Modern Physics, 75 (2003) 237
Evidence of diffusion via collective hopping in metallic supercooled liquids and glasses V. Zöllmer, K. Rätzke, F. Faupel, A. Rehmet, U. Geyer Phys. Rev. B: rapid communications, 65 (2002) 220201 (R)
Diffusion in glass-forming alloys: from the glassy state to the equilibrium melt F. Faupel, K. Rätzke, V. Zöllmer, H. Ehmler, A. Rehmet Invited review, CIMTEC 2002, 3rd Forum on new Materials, July 2002, Florence, session H: Mass and charge transport in inorganic materials, Vol.2, (2002) 171
The influence of temperature on the microstructure and mechanical properties of sputtered Cr2Nx coatings P. Kringhoj, J. Bottiger, J. Chevallier, E.J. Bienk, K. Rätzke Surface Coatings and Technology, 149 (2002) 82
7Be tracer diffusion in a deeply supercooled ZR47TI8CU7,5NI10BE27,5 melt A.Rehmet, K. Rätzke, F. Faupel, P.D. Eversheim, K. Freitag, U. Geyer S. Schneider Appl. Phys. Lett., 79 (2001) 2892
Study of oxidation behaviour of Zr based bulk amorphous alloy Zr65Cu7.5Ni0Al.5 by thermogravimetricanalyzer A.Dhawan, K. Rätzke, F. Faupel, S. K. Sharma Bulletin of Materials Science, 24 (2001) 281
Does the diffusion mechanism in thin amorphous Co81Zr19 films change during structural relaxation? A. Heesemann, K. Rätzke, V. Zöllmer, F. Faupel New Journal of Phyiscs, 3 (2001) 6.1
Does the diffusion mechanism change at the caloric glass transition of bulk metallic glasses? F. Faupel, H. Ehmler, P. Klugkist, C. Nagel, K. Rätzke L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Defect and Diffusion Forum, 194-199 (2001) 821
Chemische Zusammensetzung, Umwandlungsverhalten und mechanische Biegeeigenschaften ausgewählterkieferorthopädischer NiTi Drahtbögen M. Es-Souni, H. Fischer-Brandies, N. Kock, O. Bock, K. Rätzke Informationen aus Orthodontie und Kieferorthopädie, 33 (2001), 87
Diffusion and thermal defects in amorphous metals K. Rätzke, P. Klugkist, A. Heesemann, F. Faupel Defect and Diffusion Forum, 194-199, (2001) 833
Diffusion in metallic glasses and supercooled melts F. Faupel, K. Rätzke, H. Ehmler, P. Klugkist, V. Zöllmer, C. Nagel, A. Rehmet, A. Heesemann MRS Symp. Proc., 644 (2000) L .2.1.
Limits of ion-beam depth-profiling as used in diffusion studies of oxidation sensitive materials H. Ehmler, A. Rehmet, K. Rätzke, F. Faupel Defect and Diffusion Forum, 203-205 (2002) 147
Concentration dependence of Co diffusion in CoxZr1-x glasses A. Heesemann, K. Rätzke, V. Zöllmer, F. Faupel Z. Metallkunde, 91(2000) 909
Isotope effect of Co diffusion in thin amorphous Co51Zr49 layers during structural relaxation V. Zöllmer, H. Ehmler, K. Rätzke, P. Troche, F. Faupel Europhys. Lett., 51 (2000) 75
Evidence of highly collective Co diffusion in the whole stability range of Co-Zr glasses A. Heesemann, V. Zöllmer, K. Rätzke, F. Faupel Phys. Rev. Lett., 84 (2000) 1467
Structural effects on diffusion in metallic glasses: pressure dependence of Ni diffusion in as-quenched andrelaxed Co42Zr58 P. Klugkist, K. Rätzke, F. Faupel, P. Troche, P. Fielitz, V. Naundorf Phil. Mag. Lett., 79 (1999) 827
L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
The microstructural development of Ag/Ni multilayers during annealing K. O. Schweitz, K. Rätzke, D. Foord, A.L. Greer, H. Geisler, J. Chevallier, J. Bottiger Phil. Mag. A, 80 (2000) 1867
Positron annihilation studies of free volume changes in the bulk metallic glass Zr65Al7.5Ni10Cu17.5 duringstructural relaxation and at the glass transition C. Nagel, K. Rätzke, E. Schmidtke, Faupel, W. Ulfert Phys. Rev. B., 60 (1999) 9212
Evolution of microstructure and magnetoresistance in Cu-Co multilayers during annealing K. Rätzke, M. J. Hall. D. B. Jardine, W. C. Shi, R. E. Somekh, A. L. Greer J. Magnetism Magnetic Materials, 204 (1999) 61
Free volume changes in bulk amorphous alloys during structural relaxation and in the supercooled liquid state C. Nagel, K. Rätzke, E. Schmidtke, F. Faupel MRS Symp. Proc., 554 (1999) 75
On the role of thermal defects in diffusion in metallic glasses Defect and Diffusion Forum, 165-166 (1999) 43
Isotope effect of diffusion in the supercooled liquid state of bulk metallic glasses J. non-Cryst. sol., 250-252 (1999) 684
Evidence of defect mediated zirconium self-diffusion in amorphous Co92Zr8 Phys. Rev. Lett., 81 (1998) 614
Mass dependence of diffusion in a supercooled metallic melt H. Ehmler, A. Heesemann, K. Rätzke, F. Faupel, U. Geyer Phys. Rev. Lett., 80 (1998) 4919
Activation volume of 57Co diffusion in amorphous Co81Zr19 P. Klugkist, K. Rätzke, S. Rehders, P. Troche, F. Faupel L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Phys. Rev. Lett., 80 (1998) 3288
Free volume changes in the bulk metallic glass Zr47Ti8Cu7,5Ni10Be27,5 and the undercooled liquid C. Nagel, K. Rätzke, E. Schmidtke, J. Wolff, U. Geyer, F. Faupel Phys. Rev. B., 57 (1998) 10224
Pressure dependence of diffusion in metal-metalloid glasses invited review Proc. Joint XV International Association for the Advancement of High Pressure and Technology
& XXXIII European High Pressure Research Group Int. Conf., Warsaw, Poland, 11. - 15. 9. 1995
Pressure and mass dependence of diffusion in metallic glasses J. non-Cryst. Sol., 205-207 (1996) 607
Vanishing isotope effect of Cobalt diffusion in Fe39Ni40B21 glass J. Phys.: Cond. Matter, 7 (1995) 7663
Absence of isotope effect of diffusion in a metallic glass A. Heesemann, K. Rätzke, F. Faupel, J. Hoffmann, K. Heinemann Europhys. Lett., 29 (1995) 221
Pressure dependence of cobalt diffusion in amorphous Fe39Ni40B21 J. of non-Crys. Sol., 181 (1995) 261
Isotope effect of diffusion during structural relaxation of metallic glasses Key Engineering Materials, 81-83 (1993) 579
Highly cooperative and defect-assisted diffusion in metallic glasses Defect and Diffusion Forum, 95-98 (1993) 1175
L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Transition from single-jump type to highly cooperative diffusion during structural relaxation of a metallic glass Phys. Rev. Lett., 68 (1992) 2347
Pressure dependence of 60Co diffusion in amorphous Co76.7Fe2Nb14.3B7 Phys. Rev. B, 45 (1992) 7459
An apparatus for ion-beam sputtering and its application to high resolution radiotracer depth profiling ofdiffusion samples F. Faupel, P. W. Hüppe, K. Rätzke, R. Willecke, Th. Hehenkamp J. Vac. Sci. Technol. A, 10 (1992) 92
Pressure dependence of self diffusion in fcc cobalt at low temperature Scripta metall., 25 (1991) 2233
Pressure dependence and isotope effect of self diffusion in a metallic glass Phys. Rev. Lett., 65 (1990) 1219
L i s t o f P u b l i c a t i o n s , P r o f . D r . K l a u s R ä t z k e , K i e l
Submitted or in serious preparation condition
trimethylgermyl-1-propyne) with various geometric structure Samira M. Matson, Klaus Rätzke, Muhammad Q. Shaikh, Elena G. Litvinova, Sergey M. Shishatskiy, Klaus-Viktor Peinemann, Valeriy S. Khotimskiy submitted to Macromolecular Chemistry and Physics (5/2011)
Characterization of the spray drying behavior of emulsions containing oil droplets with a structured interface Y. Serfert, S. Drusch, J. Schröder, A. Mescher, J. Laackmann, K. Rätzke, M.Q. Shaikh and K. Schwarz Preparation and studies on polymer electrolyte composites with dispersed graphene Puja Diwan, Klaus Raetzke, Stephan Harms , Franz Faupel and Amita Chandra

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Before reAding chApter 4 Encourage speculation, but do not tell students s the answers before they read the chapter. Let them r e Before reading activities (page 44) check their own guesses as they read. The best w answers are: Activity 1 before reading s n a Activity 2 before reading s Encourage students to speculate and to make chA

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